Some VFam sets would be cool, families of all different sizes (up to 6) with furniture, pets, clothes, etc. Or maybe some toy fish for fish tycoon. What I would absolutely love is Virtual Villagers toys/collectibles (preferably collectibles), including the tree of life, huts, a lagoon (obv not real water), maybe even some food, a research table, and of course, villagers! I'm a VV girl, they're my favorite LDW games (I know I'm extremely late)
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Solving the mysteries of Isola and Margaret and Bill.